International Journal of Physics
ISSN (Print): 2333-4568 ISSN (Online): 2333-4576 Website: https://www.sciepub.com/journal/ijp Editor-in-chief: B.D. Indu
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International Journal of Physics. 2024, 12(2), 77-82
DOI: 10.12691/ijp-12-2-3
Open AccessArticle

Behavior of Atmospheric 210Pb Concentrations and Their Correlations with Meteorological Parameters in Abidjan

Gbalé G. K. Jean-Christophe1, , Adon A. Marcellin2 and Koua A. Antonin1

1Laboratory of Material Sciences, Environment, and Solar Energy, University Félix Houphouet-Boigny, Abidjan, Côte d’Ivoire

2Laboratory of Environment Sciences and Technologies, University Jean-Lorougnon Guédé, Daloa, Côte d’Ivoire

Pub. Date: April 16, 2024

Cite this paper:
Gbalé G. K. Jean-Christophe, Adon A. Marcellin and Koua A. Antonin. Behavior of Atmospheric 210Pb Concentrations and Their Correlations with Meteorological Parameters in Abidjan. International Journal of Physics. 2024; 12(2):77-82. doi: 10.12691/ijp-12-2-3

Abstract

Monitoring of radionuclides in aerosols is essential for understanding the factors influencing temporal variations in atmospheric deposition of elements such as 210Pb, which is frequently used as a tracer in atmospheric studies. However, long-term monitoring remains limited. Very few studies on air radioactivity are available in Africa and particularly in Côte d'Ivoire. In this study, we measured the radioactivity of 210Pb in surface aerosols collected on a weekly basis in the city of Abidjan in south−eastern Côte d'Ivoire from March 2022 to February 2023, using HPGe gamma spectrometry. The mean activity of 210Pb was 0.78 ± 0.2 mBq/m3. This activity concentration showed strong seasonal variations, with maximum concentrations recorded during the dry seasons and minimum in the rainy seasons. Statistically significant correlations were observed between 210Pb concentration and temperature (r = 0.47; p-value = 0.02), as well as a negative correlation with precipitation (r= -0.48; p-value = 0.02). A statistical test comparing the data obtained in the present work with some bibliographic values of 210Pb in aerosols showed that our level of activity concentration is statistically identical to the other previous studies carried out in the world. The active dependence of 210Pb with temperature and precipitation was investigated through simple linear regression analysis. Model evaluation and comparison functions were also used. Overall, this study provides an understanding of the behavior, correlations and variability of observed 210Pb concentrations influenced by atmospheric conditions in our study area.

Keywords:
210Pb Aerosol Coastal city Environmental radioactivity

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References:

[1]  Vecchi, R., Marcazzan, G. and Valli, G (2005). Seasonal variation of 210Pb activity concentration in outdoor air of Milan (Italy). J. Environ. Radioact. 82: 251–266.
 
[2]  Baskaran, M. (2011). Po-210 and Pb-210 as atmospheric tracers and global atmospheric Pb-210 fallout: A Rewiew. J. Environ. Radioact. 102: 500–513.
 
[3]  Mohan, M.P., D’Souza, R.S., Rashmi Nayak, S., Kamath, S.S. (2018). A study of temporal variations of 7Be and 210Pb concentrations and their correlations with rainfall and other parameters in the South West Coast of India. J. Environ. Radioact. 192: 194–207.
 
[4]  McNeary, D., Baskaran, M. (2003). Depositional characteristics of 7Be and 210Pb in southeastern Michigan. J. Geophys. Res. 108 (D7) 3–1-3-15.
 
[5]  Ioannidou, A., Manolopoulou, M. (2005). Temporal changes of Be-7 and Pb-210 concentrations in surface air at temperate latitudes (40°N). Appl. Radiat. Isot.63, 277–284.
 
[6]  Yu, L. (2002). Measurements of atmospheric 7Be properties using high-efficiency gamma spectroscopy. Appl. Radiat. Isot. 57, 941–946.
 
[7]  Gründel, P. (2004). Differences between the activity size distributions of the different natural radionuclide aerosols in outdoor air. Atmos. Environ. 38, 3723–3728.
 
[8]  Ali, N., Khan, E.U., Akther, P., Khattak, N.U., (2011). The effect of air mass origin on the ambient concentrations of 7Be and 210Pb in Islamabad, Pakistan. J. Environ. Radioact.102: 35-42.
 
[9]  Dekun, H., Hongyan, B., Tao, Y. (2019) Temporal Variations in Radionuclide Activity (7Be and 210Pb) in Surface Aerosols at a Coastal Site in Southeastern China,» Aerosol Air Qual. Res., 19: 1969–1979.
 
[10]  D. Afrika, 2002. [En ligne]. Available:https://discover-ivorycoast.com/climat-et-geographie/. [Acced on 23 October 2023].
 
[11]  O. Sima, D. Arnorld, C. Dovlete. (2000). Gespecor: A versatile tool in gamma-ray spectrometry. J. Radioanal. Nucl. Chem. Vol.248. No.2 359-364.
 
[12]  Team R. A language and environment for statistical computing. R Foundation for Statistical Computing,» 2022. [on line]. Available: https://www.R-project.org/..
 
[13]  Preiss, N., Mélières, M.A. and pourchet, M. (1996). A compilation of data on lead-210 concentration in surface air and fluxes at the air surface and water-sediment interfaces. J. Geophys. Res. 101: 28847–28862.
 
[14]  IAEA (2007). The environmental behaviour of polonium. In Technical reports series, International Atomic Energy Agency, Vienna.
 
[15]  E.-Y. NHO., B., Ardouin, M.F. Le Cloarec. (1996). Origins of 210Po in the atmosphere at lamto, Ivory coast: Biomass burning and saharan dust. Atmos. Environ. Vol. 30, No. 22. pp. 3705-3714.
 
[16]  Suzuki, T., maruyama, Y. Nakayama, N. (1999). Measurement of the 210Po/210Pb activity ratio in size fractionated aerosols from the coast of the Japan sea. Atmos. Environ. 33: 2285–2288.
 
[17]  Wan, G., yang, W., Shilu, W. (2005). Characteristics of U-parttern distribution of hightconcentration 210Pb in surface air at central Guizhou, China. Chin. Sci. Bull. 50: 1751–1751.
 
[18]  Eldin, M. (1971). Le climat. Abidjan, Côte d'Ivoire.
 
[19]  Feely, H.W., Larsen, R.J., Sanderson, C.G. (1998). Annual Report of the Surface Air Sampling Program: USDOE Environ. Lab, New York.
 
[20]  Kadri, I., Madis, K., and Siiri S. (2016). Lead-210 in the atmospheric air of North and South Estonia: long-term monitoring and back-trajectory calculations. Proceedings of the Estonian Academy of Sciences., 65, 4, 442-451.
 
[21]  Likuku, A.S. (2006). Factors influencing ambient concentrations of 210Pb and 7Be over the city of Edinburgh (55.9°N, 03.2°W). J. Environ. Radioact. 87, 289–304.
 
[22]  Baeza, A., Delrio, L.M., Jiminez, A., Miro, C. (1996). Analysis of the temporal evolution of atmospheric 7Be as a vector of the behaviour of other radionuclides in the atmosphere. J. Radioanal. Nucl. Chem. 207 (2), 331–334.
 
[23]  Duenas, C., Fernandez, M.C., Canete, S. and Pérez, M. (2009). 7Be and 210Pb concentration ratio in ground level air in Malaga (36.7°N, 4.5°W). Atmos. Res. 92: 49–57.
 
[24]  Pinero-Garcia, F., Ferro-Garcia, M.A., Azhara, M. (2012). 7Be behaviour in the atmosphere of the city of the Granada January 2005 to December 2009. Atmos. Environ. 47, 84-91.
 
[25]  Caillet, S., Arpagaus, P., Monna (2001). Factors controlling 7Be and 210Pb atmospheric deposition as revealed by sampling individual rain events in the region of Geneva, Switzerland. J. Environ. Radioactiv. 53, 241-256.
 
[26]  Su, C.C., Huth, C.A. and Lin, F.J. (2003). Factors controlling atmospheric fluxes of 7Be and 210Pb in northern Taiwan. Geophys.Res.Lett. 30:2018.
 
[27]  Olsen, C. L. (1985). Atmospheric fluxes and marsh-soil inventories of 7Be and 210Pb,» J. Geophys. Res 90 (6), 10487-10495.
 
[28]  Paatero, J., Buyukay, M., Holmen, K., and Viisanen, Y. (2010). Seasonal variation and source areas of airbone lead-210 at Ny-Alseund in the High Arctic. Polar Res., 29, 345–352., 2010.
 
[29]  Ahmed A. A, Mohamed, A., Ali. Seasonal variations of aerosol residence time in lower atmospheric boundary layer. J.Environ.Radioact. 77 (3), 275–283.
 
[30]  Azahra, M., Lopez-Penalver, J.J., Camacho-Garcia, M.A. (2004). Atmospheric concentrations of 7Be and 210Pb in Granada, Spain. J. Radioanal. Nucl. Chem. 261: 401–405.
 
[31]  Carvalho, F.P. (1995). Origins and concentrations of 222Rn, 210Pb, 210Bi and 210Po in the surface air at Lisbon Portugal, at the Atlantic edge of the European continental landmass. Atmos. Environ. 29: 1809–1819.
 
[32]  Sato, J., Doi, T., segawa, T. (1994). Seasonal variation of atmospheric concentrations of 210Pb and 7Be at Tsukuba, Japan, with a possible observation of 210Pb originating from the 1991 eruption of Pinatubo volcano, Philippines. Geochem. J. 28: 123–129.
 
[33]  Todorovic, D., Popovic, D., Djuric, G. ands Radenkovic, M. (2000). 210Pb in ground-level air in Belgrade city area. Atmos. Environ. 34: 3245–3248.